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W. Kirksey, H. G. Cutler, B. L. Doupnik, and J. C. Peckham, Science 179, 1324 (1973). 40. For a review of moniliformin and related cyclobutenediones see D. Bellus and H. P. Fisher, in "Advances in Pesticide S c i e n c e " (H. ), Part 2, p. 373. Pergamon, Oxford, 1979. 4 1 . G. Seitz, R. Schmiedel, and K. Mann, Arch. Pharm. ) 310, 991 (1979). 42. G. Seitz, R. Matusch, and K. -Ztg. 101, 557 (1977). 4 3 . T. Fukunaga, J. Am. Chem. Soc. 98, 610 (1976). 44. A. J. Fatiadi, Synthesis p. 165 (1978). 4 5 .

1 2 AH° 2 11 ± 1 r -26 ± 2 - 1 9 . 8 (pK = 3 . 0 5 ) 2 - 1 6 . 2 (pK = 1. SOy2 - 2 0 . /Spect. /Color. /Pot. /Pot. /Cond. /Pot. Method 6 12 16 15 36 36 21 21 25 Ref. A / / values are in kilocalories m o l e ; A S in calories m o l e K~ (entropy units); all data at 25°C. , calorimetric at ionic strength designated. For other abbreviations, seecfootnote b, Table 0I. (l Calorimetric AS" values calculated from pK values in parentheses. Calculated from data given in the reference. a 6 The Rhodizonic acid Croconic acid ~0 - 1 .

R. I. Gelb, Anal. Chem. 43, 1110 (1971). P. Souchay and M. Fleury, C. R. Hebd. Seances Acad. Sci. 252, 737 (1961). B. Carlquist and D. Dyrssen, Acta Chem. Scand. 16, 94 (1962). J. M. Carpentier, M. B. Fleury, and J. F. Verchere, Bull. Soc. Chim. Fr. 4, 1293 (1972). L. M. Schwartz, R. I. Gelb, and J. O. Yardley, J. Phys. Chem. 79, 2246 (1975). R. I. Gelb, L. M. Schwartz, D. A. Laufer, and J. O. Yardley, J. Phys. Chem. 8 1 , 1268 (1977). H. Takahashi, A. Kotaki, and K. Yagi, Seikagaku 37, 413 (1965).

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